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Identification of gallotannins and ellagitannins in aged wine spirits: a new perspective using alternative ageing technology and high-resolution mass spectrometry

2022-01-30Journal article Open access
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datacite.subject.sdg09:Indústria, Inovação e Infraestruturaspt_PT
dc.contributor.authorFernandes, Tiago
dc.contributor.authorAntunes, Alexandra M. M.
dc.contributor.authorCaldeira, Ilda
dc.contributor.authorAnjos, Ofélia
dc.contributor.authorFreitas, Victor de
dc.contributor.authorFargeton, Laurent
dc.contributor.authorBoissier, Benjamin
dc.contributor.authorCatarino, Sofia
dc.contributor.authorCanas, Sara
dc.date.accessioned2023-01-04T10:48:08Z
dc.date.available2023-01-04T10:48:08Z
dc.date.issued2022-01-30
dc.description.abstractThis research was focused on identifying gallotannins and ellagitannins degradation pathways to better understand their behavior in complex media such as wine spirits (WS). A WS was aged with chestnut wood staves with three levels of micro-oxygenation, nitrogen, and using wooden barrels. Gallotannins and ellagitannins were identified by LC-ESI-HRMS/MS using a Q-TOF in samples collected at 8, 21, 60, 180, 270, and 365 days of ageing, allowed comparing their relative abundances according to the ageing technology. It was established for the first time, the importance of oxygen in gallotannins and ellagitannins formation/degradation pathways in WS and shading light into the explanation for the steady increase of gallic and ellagic acid contents on WS during ageing. The results also highlighted the presence of penta-O-galloyl-β-D-glucose, tetra-O-galloyl-β-D-glucose, tri- O-galloyl-β-D-glucose, di-O-galloyl-β-D-glucose, and mono-O-galloyl-β-D-glucose, 2,3-(S)-hexahydroxydiphenoyl- β-D-glucose, pedunculagin, isomers vescalagin/castalagin and two products stemming from ethanol-promoted oxidation of castalagin/vescalagin and vescalin/castalin, in the composition WS aged with chestnut wood.pt_PT
dc.description.sponsorshipThis paper is a result of the research Project OXYREBRAND, funded by National Funds through FCT - Foundation for Science and Technology under the Project POCI-01-0145-FEDER-027819 (PTDC/OCE-ETA/ 27819/2017). This work was also funded by National Funds through FCT - Foundation for Science and Technology under the Projects UIDB/ 05183/2020 [MED]; UID/AGR/04129/2020, DL 57/2016/CP1382/ CT0025 [LEAF]; UIDB/00239/2020 [CEF]; UIDB/00100/2020, PTDC/ QUI-QAN/32242/2017 and UIDP/00100/2020 [CQE], and contracts CEECIND/02725/2018 (to T.A.F.) and CEECIND/02001/2017 (to A.M. M.A). Joint funding from FCT and the COMPETE Program through grant RNEM-LISBOA-01-0145-FEDER-022125 funding are also gratefully acknowledged.pt_PT
dc.description.versioninfo:eu-repo/semantics/publishedVersionpt_PT
dc.identifier.doi10.1016/j.foodchem.2022.132322pt_PT
dc.identifier.issn0308-8146
dc.identifier.urihttp://hdl.handle.net/10400.2/12972
dc.language.isoengpt_PT
dc.peerreviewedyespt_PT
dc.publisherElsevierpt_PT
dc.relationForest Research Centre
dc.relationCentro de Química Estrutural
dc.relationCentro de Química Estrutural
dc.subjectAgeing wine spiritpt_PT
dc.subjectHydrolysable tanninspt_PT
dc.subjectMicro-oxygenationpt_PT
dc.subjectChestnutpt_PT
dc.subjectMass spectrometrypt_PT
dc.titleIdentification of gallotannins and ellagitannins in aged wine spirits: a new perspective using alternative ageing technology and high-resolution mass spectrometrypt_PT
dc.typejournal article
dspace.entity.typePublication
oaire.awardTitleForest Research Centre
oaire.awardTitleCentro de Química Estrutural
oaire.awardTitleCentro de Química Estrutural
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDB%2F00239%2F2020/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDB%2F00100%2F2020/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDP%2F00100%2F2020/PT
oaire.citation.startPage132322pt_PT
oaire.citation.titleFood Chemistrypt_PT
oaire.citation.volume382pt_PT
oaire.fundingStream6817 - DCRRNI ID
oaire.fundingStream6817 - DCRRNI ID
oaire.fundingStream6817 - DCRRNI ID
person.familyNameFernandes
person.familyNamecaldeira
person.familyNameCatarino
person.familyNamede Almeida Lopes Canas
person.givenNameTiago
person.givenNameilda
person.givenNameSofia
person.givenNameSara Maria
person.identifierB-9350-2
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person.identifier.ciencia-id7212-C53B-0F02
person.identifier.ciencia-idEB11-791E-0118
person.identifier.orcid0000-0002-3374-612X
person.identifier.orcid0000-0003-2151-2008
person.identifier.orcid0000-0002-6223-4377
person.identifier.orcid0000-0002-9781-6481
person.identifier.ridB-6777-2013
person.identifier.ridB-4023-2016
person.identifier.ridD-2752-2013
person.identifier.scopus-author-id24449123500
person.identifier.scopus-author-id8056539300
person.identifier.scopus-author-id8354919700
person.identifier.scopus-author-id6507398291
project.funder.identifierhttp://doi.org/10.13039/501100001871
project.funder.identifierhttp://doi.org/10.13039/501100001871
project.funder.identifierhttp://doi.org/10.13039/501100001871
project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
rcaap.rightsopenAccesspt_PT
rcaap.typearticlept_PT
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